Microscopic Surface Structure of Liquid Alkali Metals

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Microscopic Surface Structure of Liquid Alkali Metals

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Title: Microscopic Surface Structure of Liquid Alkali Metals
Author: Tostmann, E.; DiMasi, E.; Pershan, Peter S.; Ocko, B. M.; Shpyrko, O. G.; Deutsch, M.

Note: Order does not necessarily reflect citation order of authors.

Citation: Tostmann, E., E. DiMasi, O. G. Shpyrko, Peter S. Pershan, B. M. Ocko, and M. Deutsch. 2000. Microscopic surface structure of liquid alkali metals. Physical Review B 61(11): 7284-7287.
Access Status: At the direction of the depositing author this work is not currently accessible through DASH.
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Abstract: We report an x-ray scattering study of the microscopic structure of the surface of a liquid alkali metal. The bulk liquid structure factor of the eutectic K67Na33 alloy is characteristic of an ideal mixture, and so shares the properties of an elemental liquid alkali metal. Analysis of off-specular diffuse scattering and specular x-ray reflectivity shows that the surface roughness of the K-Na alloy follows simple capillary wave behavior with a surface structure factor indicative of surface-induced layering. Comparison of the low-angle tail of the K67Na33 surface structure factor with the one measured for liquid Ga and In previously suggests that layering is less pronounced in alkali metals. Controlled exposure of the liquid to H2 and O2 gas does not affect the surface structure, indicating that oxide and hydride are not stable at the liquid surface under these experimental conditions.
Published Version: doi:10.1103/PhysRevB.61.7284
Other Sources: http://liquids.seas.harvard.edu/peter/2000.pdf/00_2_KNa.pdf
Citable link to this page: http://nrs.harvard.edu/urn-3:HUL.InstRepos:4428799

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  • FAS Scholarly Articles [7594]
    Peer reviewed scholarly articles from the Faculty of Arts and Sciences of Harvard University
 
 

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