Nanomagnetic Control of Intersystem Crossing

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Nanomagnetic Control of Intersystem Crossing

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Title: Nanomagnetic Control of Intersystem Crossing
Author: Cohen, Adam Ezra
Citation: Cohen, Adam E. 2009. Nanomagnetic control of intersystem crossing. The Journal of Physical Chemistry A 113(41): 11084-11092.
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Abstract: A theory is presented for how magnetic nanostructures can catalyze intersystem crossing in molecular radical pairs. Magnetic field gradients near physically realistic nanostructures are strong enough to induce a relative reorientation of two electronic spins in <1 ns, overwhelming nuclear hyperfine coupling as a driver of intersystem crossing. Nanomagnetic control of intersystem crossing represents a form of heterogeneous catalysis that does not require molecular contact, but only short-range magnetic coupling.
Published Version: doi:10.1021/jp907113p
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