| Title: | Probing Biological Light-Harvesting Phenomena by Optical Cavities |
| Author: |
Caruso, Filippo; Saikin, Semion K.; Solano, Enrique; Aspuru-Guzik, Alán; Plenio, Martin B.; Huelga, Susana F.
Note: Order does not necessarily reflect citation order of authors. |
| Citation: | Caruso, Filippo, Semion K. Saikin, Enrique Solano, Susana F. Huelga, Alán Aspuru-Guzik, and Martin B. Plenio. 2012. Probing biological light-harvesting phenomena by optical cavities. Physical Review B 85(12): 125424. |
| Full Text & Related Files: |
Probing_biological_lightharvesting.pdf (7.076Mb; PDF)
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| Abstract: | We propose a driven optical cavity quantum electrodynamics (QED) setup aimed at directly probing energy transport dynamics in photosynthetic biomolecules. We show that detailed information concerning energy transfer paths and delocalization of exciton states can be inferred (and exciton energies estimated) from the statistical properties of the emitted photons. This approach provides us with a spectroscopic tool to interrogate biological systems in terms of quantum optical phenomena which have usually been studied in solid-state or atomic systems (e.g., semiconductor quantum dots and trapped atoms) and which are now extended to a broader range of spectroscopy experiments. |
| Published Version: | doi:10.1103/PhysRevB.85.125424 |
| Other Sources: | http://arxiv.org/abs/1110.1386 |
| Terms of Use: | This article is made available under the terms and conditions applicable to Open Access Policy Articles, as set forth at http://nrs.harvard.edu/urn-3:HUL.InstRepos:dash.current.terms-of-use#OAP |
| Citable link to this page: | http://nrs.harvard.edu/urn-3:HUL.InstRepos:8641796 |
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