Now showing items 1-6 of 6

• #### A Correlated-Polaron Electronic Propagator: Open Electronic Dynamics beyond the Born-Oppenheimer Approximation ﻿

(American Institute of Physics, 2012)
In this work, we develop an approach to treat correlated many-electron dynamics, dressed by the presence of a finite-temperature harmonic bath. Our theory combines a small polaron transformation with the second-order ...
• #### Exciton Coherence Lifetimes from Electronic Structure ﻿

(American Institute of Physics, 2012-04-06)
We model the coherent energy transfer of an electronic excitation within covalently linked aromatic homodimers from first-principles. Our results shed light on whether commonly used models of the bath calculated via detailed ...

• #### Measurement of the Third-Order Nonlinear Optical Susceptibility $\chi^{(3)}$ for the $1002-cm^{-1}$ Mode of Benzenethiol Using Coherent Anti-Stokes Raman Scattering with Continuous-Wave Diode Lasers ﻿
The components of the third-order nonlinear optical susceptibility $\chi^{(3)}$ for the $1002-cm^{–1}$ mode of neat benzenethiol have been measured using coherent anti-Stokes Raman scattering with continuous-wave diode ...