Quantum process tomography by 2D fluorescence spectroscopy

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Quantum process tomography by 2D fluorescence spectroscopy

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Title: Quantum process tomography by 2D fluorescence spectroscopy
Author: Pachón, Leonardo A.; Marcus, Andrew H.; Aspuru-Guzik, Alan

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Citation: Pachón, Leonardo A., Andrew H. Marcus, and Alán Aspuru-Guzik. 2015. “Quantum Process Tomography by 2D Fluorescence Spectroscopy.” J. Chem. Phys. 142 (21) (June 7): 212442. Portico. doi:10.1063/1.4919954.
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Abstract: Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter Γ of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications to foundational and applied problems, as well as further extensions, are discussed.
Published Version: doi:10.1063/1.4919954
Other Sources: http://arxiv.org/pdf/1502.02363v2.pdf
Terms of Use: This article is made available under the terms and conditions applicable to Open Access Policy Articles, as set forth at http://nrs.harvard.edu/urn-3:HUL.InstRepos:dash.current.terms-of-use#OAP
Citable link to this page: http://nrs.harvard.edu/urn-3:HUL.InstRepos:23670486
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