Yao, Norman YBintz, Marcus2026-06-0920262026-05-142026Bintz, Marcus. 2026. Quantum Magnetism in Dipolar Rydberg Atom Arrays. Doctoral Dissertation, Harvard University Graduate School of Arts and Sciences.32702644https://dash.harvard.edu/handle/1/42740455This thesis demonstrates that arrays of electric dipoles are good analogs for quantum magnets. We center our investigation on a recently developed experiment, in which rubidium-87 atoms are trapped in optical tweezers and then excited into two distinct electronic Rydberg states. The electric dipole-dipole interaction between these Rydberg atoms is mathematically modeled by a spin Hamiltonian with easy-plane anisotropy, and coupling strength decaying as the inverse cube of the distance. We approximately solve for the ground state of this model Hamiltonian on each of the eleven Archimedean lattices, through large-scale density matrix renormalization group calculations. For the kagome lattice, we gather extensive numerical evidence for an emergent quantum spin liquid, similar to that occurring in the canonical Heisenberg model of quantum magnetism. We predict this spin liquid to be of 𝑈(1) Dirac type, and propose new protocols for experimentally preparing and characterizing it. Our theoretical calculations support the collaborative design and analysis of experiments studying dipolar Rydberg atoms in square, circular, and kagome arrays. These respectively result in observations of continuous symmetry breaking, Tomonaga-Luttinger liquid behavior, and an atomic spin liquid candidate.application/pdfenPhysicsThesis or Dissertation2026-06-090000-0002-4548-3953