Person:

Medford, James Redding

Quantum-dot spin qubits characteristically use oscillating magnetic or electric fields, or quasi-static Zeeman field gradients, to realize full qubit control. For the case of three confined electrons, exchange interaction between two pairs allows qubit rotation around two axes, hence full control, using only electrostatic gates. Here, we report initialization, full control, and single-shot readout of a three-electron exchange-driven spin qubit. Control via the exchange interaction is fast, yielding a demonstrated 75 qubit rotations in less than 2 ns. Measurement and state tomography are performed using a maximum-likelihood estimator method, allowing decoherence, leakage out of the qubit state space, and measurement fidelity to be quantified. The methods developed here are generally applicable to systems with state leakage, noisy measurements and non-orthogonal control axes.

Using single-shot charge detection in a GaAs double quantum dot, we investigate spin relaxation time (T1) and readout visibility of a two-electron singlet-triplet qubit following single-electron dynamic nuclear polarization (DNP). For magnetic fields up to 2 T, the DNP cycle is in all cases found to increase Overhauser field gradients, which in turn decrease T1 and, consequently, reduce readout visibility. This effect was previously attributed to a suppression of singlet-triplet dephasing under a similar DNP cycle. A model describing relaxation after singlet-triplet mixing agrees well with experiment. Effects of pulse bandwidth on visibility are also investigated.

This thesis presents research on the initialization, control, and readout of electron spin states in gate defined GaAs quantum dots. The first three experiments were performed with Singlet-Triplet spin qubits in double quantum dots, while the remaining two experiments were performed with an Exchange-Only spin qubit in a triple quantum dot.

Single-shot measurement of the charge arrangement and spin state of a double quantum dot are reported with measurement times down to 100 ns. Sensing uses radio-frequency reflectometry of a proximal quantum dot in the Coulomb blockade regime. The sensor quantum dot is up to 30 times more sensitive than a comparable quantum point-contact sensor and yields three times greater signal to noise in rf single-shot measurements. Numerical modeling is qualitatively consistent with experiment and shows that the improved sensitivity of the sensor quantum dot results from reduced lifetime broadening and screening.

We introduce a solid-state qubit in which exchange interactions among confined electrons provide both the static longitudinal field and the oscillatory transverse field, allowing rapid and full qubit control via rf gate-voltage pulses. We demonstrate two-axis control at a detuning sweet spot, where leakage due to hyperfine coupling is suppressed by the large exchange gap. A π/2-gate time of 2.5 ns and a coherence time of 19  μs, using multipulse echo, are also demonstrated. Model calculations that include effects of hyperfine noise are in excellent quantitative agreement with experiment.