Person:

Komar, Peter

We describe how strong resonant interactions in multimode optomechanical systems can be used to induce controlled nonlinear couplings between single photons and phonons. Combined with linear mapping schemes between photons and phonons, these techniques provide a universal building block for various classical and quantum information processing applications. Our approach is especially suited for nano-optomechanical devices, where strong optomechanical interactions on a single photon level are within experimental reach.

We present a detailed theoretical analysis of a weakly driven, multimode optomechanical system, in which two optical modes are strongly and near-resonantly coupled to a single mechanical mode via a three-wave mixing interaction. We calculate one- and two-time intensity correlations of the two optical fields and compare them to analogous correlations in atom-cavity systems. Nonclassical photon correlations arise when the optomechanical coupling g exceeds the cavity decay rate κ, and we discuss signatures of one- and two-photon resonances as well as quantum interference. We also find a long-lived correlation that decays slowly with the mechanical decay rate γ, reflecting the heralded preparation of a single-phonon state after detection of a photon. Our results provide insight into the quantum regime of multimode optomechanics, with potential applications for quantum information processing with photons and phonons.

We present a quantum-enhanced atomic clock protocol based on groups of sequentially larger Greenberger-Horne-Zeilinger (GHZ) states that achieves the best clock stability allowed by quantum theory up to a logarithmic correction. Importantly the protocol is designed to work under realistic conditions where the drift of the phase of the laser interrogating the atoms is the main source of decoherence. The simultaneous interrogation of the laser phase with a cascade of GHZ states realizes an incoherent version of the phase estimation algorithm that enables Heisenberg-limited operation while extending the coherent interrogation time beyond the laser noise limit. We compare and merge the new protocol with existing state of the art interrogation schemes, and identify the precise conditions under which entanglement provides an advantage for clock stabilization: it allows a significant gain in the stability for short averaging time.

We propose and analyze heralded quantum gates between qubits in optical cavities. They employ an auxiliary qubit to report if a successful gate occurred. In this manner, the errors, which would have corrupted a deterministic gate, are converted into a nonunity probability of success: once successful, the gate has a much higher fidelity than a similar deterministic gate. Specifically, we describe that a heralded, near-deterministic controlled phase gate (CZ gate) with the conditional error arbitrarily close to zero and the success probability that approaches unity as the cooperativity of the system, C, becomes large. Furthermore, we describe an extension to near-deterministic N-qubit Toffoli gate with a favorable error scaling. These gates can be directly employed in quantum repeater networks to facilitate near-ideal entanglement swapping, thus greatly speeding up the entanglement distribution.

Individual atoms in optical cavities can provide an efficient interface between stationary qubits and flying qubits (photons), which is an essential building block for quantum communication. Furthermore, cavity-assisted controlled-not (cnot) gates can be used for swapping entanglement to long distances in a quantum repeater setup. Nonetheless, dissipation introduced by the cavity during the cnot may increase the experimental difficulty in obtaining long-distance entanglement distribution using these systems. We analyze and compare a number of cavity-based repeater schemes combining various entanglement generation schemes and cavity-assisted cnot gates. We find that a scheme, where high-fidelity entanglement is first generated in a two-photon detection scheme and then swapped to long distances using a recently proposed heralded controlled-Z (cz) gate, exhibits superior performance compared to the other schemes. The heralded gate moves the effect of dissipation from the fidelity to the success probability of the gate thereby enabling high-fidelity entanglement swapping. As a result, high-rate entanglement distribution can be achieved over long distances even for low cooperativities of the atom-cavity systems. This high-fidelity repeater is shown to outperform the other cavity-based schemes by up to two orders of magnitude in the rate for realistic parameters and large distances (1000 km).

We study the effect of resonances associated with complex molecular interaction of Rydberg atoms on Rydberg blockade. We show that densely spaced molecular potentials between doubly excited atomic pairs become unavoidably resonant with the optical excitation at short interatomic separations. Such molecular resonances limit the coherent control of individual excitations in Rydberg blockade. As an illustration, we compute the molecular interaction potentials of Rb atoms near the 100s states asymptote to characterize such detrimental molecular resonances and determine the resonant loss rate to molecules and inhomogeneous light shifts. Techniques to avoid the undesired effect of molecular resonances are discussed.

The current frontier of our understanding of the physical universe is dominated by quantum phenomena. Uncovering the prospects and limitations of acquiring and processing information using quantum effects is an outstanding challenge in physical science. This thesis presents an analysis of several new model systems and applications for quantum information processing and metrology.

First, we analyze quantum optomechanical systems exhibiting quantum phenomena in both optical and mechanical degrees of freedom. We investigate the strength of non-classical correlations in a model system of two optical and one mechanical mode. We propose and analyze experimental protocols that exploit these correlations for quantum computation.

We then turn our attention to atom-cavity systems involving strong coupling of atoms with optical photons, and investigate the possibility of using them to store information robustly and as relay nodes. We present a scheme for a robust two-qubit quantum gate with inherent error-detection capabilities. We consider several remote entanglement protocols employing this robust gate, and we use these systems to study the performance of the gate in practical applications.

Finally, we present a new protocol for running multiple, remote atomic clocks in quantum unison. We show that by creating a cascade of independent Greenberger-Horne-Zeilinger states distributed across the network, the scheme asymptotically reaches the Heisenberg limit, the fundamental limit of measurement accuracy. We propose an experimental realization of such a network consisting of neutral atom clocks, and analyze the practical performance of such a system.