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Gelly, Ryan

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Gelly

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Ryan

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Gelly, Ryan
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    An Inverse-Designed Nanophotonic Interface for Excitons in Atomically Thin Materials
    (American Chemical Society (ACS), 2023-09-11) Gelly, Ryan; White, Alexander; Scuri, Giovanni; Liao, Xing; Geun Ho, Ahn; Deng, Bingchen; Watanabe, Kenji; Taniguchi, Takashi; Vučković, Jelena; Park, Hongkung
    Efficient nanophotonic devices are essential for applications in quantum networking, optical information processing, sensing, and nonlinear optics. Extensive research efforts have focused on integrating two-dimensional (2D) materials into photonic structures, but this integration is often limited by size and material quality. Here, we use hexagonal boron nitride (hBN), a benchmark choice for encapsulating atomically thin materials, as a waveguiding layer while simultaneously improving the optical quality of the embedded films. When combined with photonic inverse design, it becomes a complete nanophotonic platform to interface with optically active 2D materials. Grating couplers and low-loss waveguides provide optical interfacing and routing, tunable cavities provide a large exciton-photon coupling to transition metal dichalcogenides (TMD) monolayers through Purcell enhancement, and metasurfaces enable the efficient detection of TMD dark excitons. This work paves the way for advanced 2D-material nanophotonic structures for classical and quantum nonlinear optics.
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    Broken Mirror Symmetry in Excitonic Response of Reconstructed Domains in Twisted MoSe2/MoSe2 Bilayers
    (Springer Science and Business Media LLC, 2020-07-13) Sung, Jiho; Zhou, You; Scuri, Giovanni; Zólyomi, Viktor; Andersen, Trond; Yoo, Hyobin; Wild, Dominik; Joe, Andrew Y.; Gelly, Ryan; Heo, Hoseok; Magorrian, Samuel J.; Berube, Damien; Valdivia, Andrés M. Mier; Taniguchi, Takashi; Watanabe, Kenji; Lukin, Mikhail D.; Kim, Philip; Fal’ko, Vladimir I.; Park, Hongkun
    Van der Waals heterostructures obtained via stacking and twisting have been used to create moiré superlattices, enabling new optical and electronic properties in solid-state systems. Moiré lattices in twisted bilayers of transition metal dichalcogenides (TMDs) result in exciton trapping, host Mott insulating and superconducting states, and act as unique Hubbard systems whose correlated electronic states can be detected and manipulated optically. Structurally, these twisted heterostructures feature atomic reconstruction and domain formation. However, due to the nanoscale sizes of moiré domains, the effects of atomic reconstruction on the electronic and excitonic properties could not be systematically investigated. Here, we use near 0o twist angle MoSe2/MoSe2 bilayers with large rhombohedral AB/BA domains to directly probe excitonic properties of individual domains with far-field optics. We show that this system features broken mirror/inversion symmetry, with the AB and BA domains supporting interlayer excitons with out-of-plane electric dipole moments in opposite directions. The dipole orientation of ground-state Γ-K interlayer excitons can be flipped with electric fields, while higher-energy K-K interlayer excitons undergo field-asymmetric hybridization with intralayer K-K excitons. Our study reveals the impact of crystal symmetry on TMD excitons and points to new avenues for realizing topologically nontrivial systems, exotic metasurfaces, collective excitonic phases, and quantum emitter arrays via domain-pattern engineering.