Cavity electro-optics in thin-film lithium niobate

Abstract

Quantum networks of superconducting qubits linked by optical channels could leverage both the quantum information processing capabilities of superconducting circuits and the long communication distances provided by optical photons. Such networks would require high efficiency, low noise, and wide bandwidth transducers between microwave and optical frequencies. Transducers based on the Pockels electro-optic (EO) effect are particularly promising in this application for their direct conversion mechanism and potential for strong performance. EO transducers could also be used for sensitive optical modulators and low-noise detection of microwave and millimeter-wave signals. This dissertation presents recent work to create cavity EO transducers in thin-film lithium niobate, an integrated photonics platform that provides low optical loss and strong EO coupling. I first describe the theory of cavity electro-optics and how it can be used to generate high-efficiency transduction between microwave and optical fields. An initial device is presented and characterized, demonstrating per-photon on-chip transduction efficiencies of up to (2.7 ± 0.3) × 10^−5. A key benefit of the device described here, which is based on photonic molecule modes, is the ability to use a static electro-optic bias to trim the transducer into resonance. However, we find the migration of free carriers in thin-film lithium niobate reduces the EO response of the device to static fields, making such trimming ineffective. This carrier migration is a key challenge for enabling the promise of low-power electro-optics provided by thin-film lithium niobate devices. I characterize the low-frequency electro-optic response, which suggests that conduction occurs on the etched surface of lithium niobate. I show how this conduction can be reduced – and low-frequency EO performance improved – by changing the electrode design and annealing the devices. Following this, I describe the design and initial characterization of an improved transducer device. Finally, I describe a scheme by which even relatively low-efficiency transducers could be used to generate remote entanglement using an optically heralding scheme. Demonstration of such a system appears possible with current devices, suggesting that small opticallymediated quantum networks of superconducting qubits may be feasible soon.