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Topological and symmetry-breaking phases of strongly correlated systems: From quantum materials to ultracold atoms

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2022-05-19

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Samajdar, Rhine. 2022. Topological and symmetry-breaking phases of strongly correlated systems: From quantum materials to ultracold atoms. Doctoral dissertation, Harvard University Graduate School of Arts and Sciences.

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The physics of strongly interacting particles is often extraordinarily rich, leading to the \textit{emergence} of fundamentally new phases and phenomena that cannot exist in the absence of correlations. This thesis is devoted to the study of different classes of quantum systems with such strong correlations.

Programmable quantum simulators based on Rydberg atom arrays have recently emerged as versatile platforms to probe quantum many-body phases and their dynamics. In Chapter 2, we start with theories of quantum phase transitions (QPTs) in one-dimensional chains of Rydberg atoms. We demonstrate the existence of a novel QPT in the universality class of the $\mathbb{Z}^{}_3$ chiral clock model, calculate its critical exponents, and discuss their measurement with the quantum Kibble-Zurek mechanism. Proceeding to two dimensions, Chapter 3 describes the zero-temperature phase diagram of a square-lattice Rydberg atom array, revealing several experimentally realizable density-wave-ordered phases and QPTs. For a different geometry, namely, the kagome lattice studied in Chapter 4, we identify a regime that constitutes a likely candidate for hosting a phase with long-range quantum entanglement and topological order. Based on mappings to dimer models and gauge theories, we argue for the existence of a quantum spin liquid phase that has proved elusive in solid-state materials.

In the next part of this thesis, we focus on similarly strongly correlated phases in the realm of quantum materials. Motivated by recent observations of an enhanced thermal Hall response in the high-temperature cuprate superconductors, in Chapter 5, we study the thermal Hall conductivity, $\kappa^{}{xy}$, of chiral spin-liquid ans"{a}tze on the square lattice, focusing on the contribution from neutral (bosonic or fermionic) spinons. Thereafter, going beyond mean-field theory, we consider the corrections due to emergent gauge fields, which yield a response of opposite sign to that of the fermionic matter. We additionally consider the contribution of phonons to $\kappa^{}{xy}$ and establish its relation to the spinon Hall viscosity. Thermal Hall measurements also leave intriguing fingerprints in Kitaev materials like $\alpha$-RuCl$3$, and in this context, Chapter 6 investigates the unquantized $\kappa{xy}$ obtained in a gapless spinon Fermi surface state.

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Cuprates, Gauge theory, Quantum simulation, Quantum spin liquids, Rydberg atoms, Thermal Hall effect, Physics, Condensed matter physics, Atomic physics

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