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A room temperature low-threshold ultraviolet plasmonic nanolaser

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2014

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Nature Publishing Group
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Zhang, Qing, Guangyuan Li, Xinfeng Liu, Fang Qian, Yat Li, Tze Chien Sum, Charles M. Lieber, and Qihua Xiong. 2014. “A Room Temperature Low-Threshold Ultraviolet Plasmonic Nanolaser.” Nature Communications 5: 4953.

Abstract

Constrained by large ohmic and radiation losses, plasmonic nanolasers operated at visible regime are usually achieved either with a high threshold (102–104 MW cm−2) or at cryogenic temperatures (4–120 K). Particularly, the bending-back effect of surface plasmon (SP) dispersion at high energy makes the SP lasing below 450 nm more challenging. Here we demonstrate the first strong room temperature ultraviolet (~370 nm) SP polariton laser with an extremely low threshold (~3.5 MW cm−2). We find that a closed-contact planar semiconductor–insulator–metal interface greatly lessens the scattering loss, and more importantly, efficiently promotes the exciton–SP energy transfer thus furnishes adequate optical gain to compensate the loss. An excitation polarization-dependent lasing action is observed and interpreted with a microscopic energy-transfer process from excitons to SPs. Our work advances the fundamental understanding of hybrid plasmonic waveguide laser and provides a solution of realizing room temperature UV nanolasers for biological applications and information technologies.

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Physical sciences, Optical physics

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