Publication:
Quantum Dynamics of a Particle Interacting with Lattice Vibrations and Disorder Potentials

No Thumbnail Available

Date

2023-07-25

Published Version

Published Version

Journal Title

Journal ISSN

Volume Title

Publisher

The Harvard community has made this article openly available. Please share how this access benefits you.

Research Projects

Organizational Units

Journal Issue

Citation

Kim, Donghwan. 2023. Quantum Dynamics of a Particle Interacting with Lattice Vibrations and Disorder Potentials. Doctoral dissertation, Harvard University Graduate School of Arts and Sciences.

Research Data

Abstract

Understanding the fundamental behavior of matter requires studying the quantum dynamics of a particle interacting with lattice vibrations and disorder potentials. In the first part of this dissertation, lattice vibrations are represented using the coherent state representation, resulting in a quasiclassical field that serves as a dynamic disorder potential for a particle. The dynamics of the particle within this potential are treated nonperturbatively to preserve coherence beyond single collision events. This approach is effective in capturing particle coherence effects and computing the density of states. Specifically, the low-energy tail of the spectral density is calculated and its relationship to static disorder potentials is established in the classical phonon limit. In the second part of the dissertation, it is shown that even in the absence of periodic structure in a static disorder potential, sharp Bragg diffraction of the wave is still observed. This phenomenon resembles a powder diffraction pattern but includes nontrivial partially resonant scattering that violates Fermi’s golden rule.

Description

Other Available Sources

Keywords

Chemistry, Physical chemistry, Physics

Terms of Use

This article is made available under the terms and conditions applicable to Other Posted Material (LAA), as set forth at Terms of Service

Endorsement

Review

Supplemented By

Referenced By

Related Stories