Person:

Diehl, L

In this study, we report the unequivocal demonstration of midinfrared mode-locked pulses from quantum cascade lasers. The train of short pulses was generated by actively modulating the current and hence the gain of an edge-emitting quantum cascade laser (QCL). Pulses with duration of about 3 ps at full-width-at-half-maxima and energy of 0.5 pJ were characterized using a second-order interferometric autocorrelation technique based on a nonlinear quantum well infrared photodetector. The mode-locking dynamics in the QCLs was modeled based on the Maxwell-Bloch equations in an open two-level system. Our model reproduces the overall shape of the measured autocorrelation traces and predicts that the short pulses are accompanied by substantial wings as a result of strong spatial hole burning. The range of parameters where short mode-locked pulses can be formed is found.

An ultra-broadband distributed-feedback quantum cascade laser array was fabricated, using a heterogeneous cascade based on two bound-to-continuum designs centered at 8.4 and 9.6 mum. This array emitted in a range over 220 cm-1 near a 9-mu m wavelength, operated in pulsed mode at room temperature. The output power of the array varied between 100- and 1100-mW peak intensity.

We report experimental demonstration of directional light emission from limaçon-shaped microcavity semiconductor lasers. Quantum cascade lasers (QCLs) emitting at (\lambda \approx 10 \mu m) are used as a model system. Both ray optics and wave simulations show that for deformations in the range (0.37< \epsilon <0.43), these microcavities support high quality-factor whispering gallerylike modes while having a directional far-field profile with a beam divergence (\theta \approx 30°) in the plane of the cavity. The measured far-field profiles are in good agreement with simulations. While the measured spectra show a transition from whispering gallerylike modes to a more complex mode structure at higher pumping currents, the far field is insensitive to the pumping current demonstrating the predicted “universal far-field behavior” of this class of chaotic resonators. Due to their relatively high quality factor, our microcavity lasers display reduced threshold current densities compared to conventional ridge lasers with millimeter-long cavities. The performance of the limaçon-shaped QCLs is robust with respect to variations of the deformation near its optimum value of ( \epsilon = 0.40).

DFB quantum cascade laser (DFB-QCL) arrays operating between 8.7 and 9.4 mum are investigated for their performance characteristics-single-mode selection of the DFB grating, and variability in threshold, slope efficiency, and output power of different lasers in the array. Single-mode selection refers to the ability to choose a desired mode/frequency of laser emission with a DFB grating. We apply a theoretical framework developed for general DFB gratings to analyze DFB-QCL arrays. We calculate how the performance characteristics of DFB-QCLs are affected by the coupling strength kappaL of the grating, and the relative position of the mirror facets at the ends of the laser cavity with respect to the grating. We discuss how single-mode selection can be improved by design. Several DFB-QCL arrays are fabricated and their performance examined. We achieve desired improvements in single-mode selection, and we observe the predicted variability in the threshold, slope efficiency, and output power of the DFB-QCLs. As a demonstration of potential applications, the DFB-QCL arrays are used to perform infrared absorption spectroscopy with fluids.