Person:

Halperin, Bertrand

The central-spin problem is a widely studied model of quantum decoherence. Dynamic nuclear polarization occurs in central-spin systems when electronic angular momentum is transferred to nuclear spins and is exploited in quantum information processing for coherent spin manipulation. However, the mechanisms limiting this process remain only partially understood. Here we show that spin–orbit coupling can quench dynamic nuclear polarization in a GaAs quantum dot, because spin conservation is violated in the electron–nuclear system, despite weak spin–orbit coupling in GaAs. Using Landau–Zener sweeps to measure static and dynamic properties of the electron spin–flip probability, we observe that the size of the spin–orbit and hyperfine interactions depends on the magnitude and direction of applied magnetic field. We find that dynamic nuclear polarization is quenched when the spin–orbit contribution exceeds the hyperfine, in agreement with a theoretical model. Our results shed light on the surprisingly strong effect of spin–orbit coupling in central-spin systems.

Inspired by the creation of a fast exchange-only qubit [Medford et al., Phys. Rev. Lett. 111, 050501 (2013)], we develop a theory describing the nonlinear dynamics of two such qubits that are capacitively coupled, when one of them is driven resonantly at a frequency equal to its level splitting. We include conditions of strong driving, where the Rabi frequency is a significant fraction of the level splitting, and we consider situations where the splitting for the second qubit may be the same as or different than the first. We demonstrate that coupling between qubits can be detected by reading the response of the second qubit, even when the coupling between them is only of about 1% of their level splittings, and we calculate entanglement between qubits. Patterns of nonlinear dynamics of coupled qubits and their entanglement are strongly dependent on the geometry of the system, and the specific mechanism of interqubit coupling deeply influences dynamics of both qubits. In particular, we describe the development of irregular dynamics in a two-qubit system, explore approaches for inhibiting it, and demonstrate the existence of an optimal range of coupling strength maintaining stability during the operational time.

We develop a theory of extrinsic spin currents in semiconductors, resulting from spin-orbit coupling at charged scatterers, which leads to skew-scattering and side-jump contributions to the spin-Hall conductivity. Applying the theory to bulk n-GaAs, without any free parameters, we find spin currents that are in reasonable agreement with experiments by Kato et al.

Spin polarization may be generated far from the boundaries of a sample by nonlinear effects of an electric current, in the presence of "extrinsic" spin-orbit interactions, even when such generation is forbidden in the linear regime. We present a Corbino model where spin accumulation results from a combination of current gradients, nonlinearity, and cubic anisotropy. Further, we show that even with isotropic conductivity, nonlinear effects in a low-symmetry sidearm geometry can generate spin polarization far away from boundaries. Finally, we find that drift from the boundaries dominates spin polarization patterns observed in recent experiments on GaAs by Sih et al. [Phys. Rev. Lett. 97, 096605 (2006)].

Spin Hall effects are a collection of phenomena, resulting from spin-orbit coupling, in which an electrical current flowing through a sample can lead to spin transport in a perpendicular direction and spin accumulation at lateral boundaries. These effects, which do not require an applied magnetic field, can originate in a variety of intrinsic and extrinsic spin-orbit coupling mechanisms and depend on geometry, dimension, impurity scattering, and carrier density of the system—making the analysis of these effects a diverse field of research. In this chapter, we give an overview of the theoretical background of the spin Hall effects and summarize some of the most important results. First, we explain effective spin-orbit Hamiltonians, how they arise from band structure, and how they can be understood from symmetry considerations; including intrinsic coupling due to bulk inversion or structure asymmetry or due to strain, and extrinsic coupling due to impurities. This leads to different mechanisms of spin transport: spin precession, skew scattering, and side jump. Then we present the kinetic (Boltzmann) equations, which describe the spin-dependent distribution function of charge carriers, and the diffusion equation for spin-polarization density. Next, we define the notion of spin currents and discuss their relation to spin polarization. Finally, we explain the electrically induced spin effects; namely, spin polarization and currents in bulk and near boundaries (the focus of most current theoretical research efforts), and spin injection, as well as effects in mesoscopic systems and in edge states.

We investigate capacitively-coupled exchange-only two-qubit quantum gates based on quantum dots. For exchange-only coded qubits electron spin S and its projection Sz are exact quantum numbers. Capacitive coupling between qubits, as distinct from interqubit exchange, preserves these quantum numbers. We prove, both analytically and numerically, that conservation of the spins of individual qubits has a dramatic effect on the performance of two-qubit gates. By varying the level splittings of individual qubits, Ja and Jb, and the interqubit coupling time, t, we can find an infinite number of triples (Ja,Jb,t) for which the two-qubit entanglement, in combination with appropriate single-qubit rotations, can produce an exact cnot gate. This statement is true for practically arbitrary magnitude and form of capacitive interqubit coupling. Our findings promise a large decrease in the number of nonlocal (two-qubit) operations in quantum circuits.

We present experimental data and associated theory for correlations in a series of experiments involving repeated Landau-Zener sweeps through the crossing point of a singlet state and a spin-aligned triplet state in a GaAs double quantum dot containing two conduction electrons, which are loaded in the singlet state before each sweep, and the final spin is recorded after each sweep. The experiments reported here measure correlations on time scales from 4 μs to 2 ms. When the magnetic field is aligned in a direction such that spin-orbit coupling cannot cause spin flips, the correlation spectrum has prominent peaks centered at zero frequency and at the differences of the Larmor frequencies of the nuclei, on top of a frequency-independent background. When the spin-orbit field is relevant, there are additional peaks, centered at the frequencies of the individual species. A theoretical model which neglects the effects of high-frequency charge noise correctly predicts the positions of the observed peaks, and gives a reasonably accurate prediction of the size of the frequency-independent background, but gives peak areas that are larger than the observed areas by a factor of 2 or more. The observed peak widths are roughly consistent with predictions based on nuclear dephasing times of the order of 60 μs. However, there is extra weight at the lowest observed frequencies, which suggests the existence of residual correlations on the scale of 2 ms. We speculate on the source of these discrepancies.