Person:

Taylor, Jacob

We theoretically investigate the controlled dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. Three regimes of long-term dynamics are identified, including the buildup of a large difference in the Overhauser fields across the dots, the saturation of the nuclear polarization process associated with formation of so-called ‘‘dark states’’, and the elimination of the difference field. We show that in the case of unequal dots, buildup of difference fields generally accompanies the nuclear polarization process, whereas for nearly identical dots, buildup of difference fields competes with polarization saturation in dark states. The elimination of the difference field does not, in general, correspond to a stable steady state of the polarization process.

The influence of gate-controlled two-electron exchange on the relaxation of nuclear polarization in small ensembles ((N \sim 10^6)) of nuclear spins is examined in a GaAs double quantum dot system. Waiting in the (2,0) charge configuration, which has large exchange splitting, reduces the nuclear diffusion rate compared to that of the (1,1) configuration. Matching exchange to Zeeman splitting significantly increases the nuclear diffusion rate.

Initialization, two-spin coherent manipulation, and readout of a three-spin qubit are demonstrated using a few-electron triple quantum dot. The three-spin qubit is designed to allow all operations for full qubit control to be tuned via nearest-neighbor exchange interaction. Fast readout of charge states takes advantage of multiplexed reflectometry. Decoherence measured in a two-spin subspace is found to be consistent with predictions based on gate voltage noise with a uniform power spectrum. The theory of the exchange-only qubit is developed and it is shown that initialization of only two spins suffices for operation. Requirements for full multiqubit control using only exchange and electrostatic interactions are outlined.